Selective-exhaust gas recirculation for CO2 capture using membrane technology

dc.contributor.authorRusso, Giuseppe
dc.contributor.authorPrpich, George
dc.contributor.authorAnthony, Edward J.
dc.contributor.authorMontagnaro, Fabio
dc.contributor.authorJurado Pontes, Nelia
dc.contributor.authorDi Lorenzo, Giuseppina
dc.contributor.authorDarabkhani, Hamidreza Gohari
dc.date.accessioned2017-11-14T09:33:07Z
dc.date.available2017-11-14T09:33:07Z
dc.date.issued2017-11-10
dc.description.abstractMembranes can potentially offer low-cost CO2 capture from post-combustion flue gas. However, the low partial pressure of CO2 in flue gases can inhibit their effectiveness unless methods are employed to increase their partial pressure. Selective-Exhaust Gas Recirculation (S-EGR) has recently received considerable attention. In this study, the performance of a dense polydimethylsiloxane (PDMS) membrane for the separation of CO2/N2 binary model mixtures for S-EGR application was investigated using a bench-scale experimental rig. Measurements at different pressures, at different feeding concentrations and with nitrogen as sweep gas revealed an average carbon dioxide permeability of 2943 ± 4.1%RSD Barrer. The bench-scale membrane module showed high potential to separate binary mixtures of N2 and CO2 containing 5–20% CO2. The permeability was slightly affected by feed pressures ranging from 1 to 2.4 bar. Furthermore, the separation selectivity for a CO2/N2 mixture of 10%/90% (by volume) reached a maximum of 10.55 at 1.8 bar. Based on the results from the bench-scale experiments, a pilot-scale PDMS membrane module was tested for the first time using a real flue gas mixture taken from the combustion of natural gas. Results from the pilot-scale experiments confirmed the potential of the PDMS membrane system to be used in an S-EGR configuration for capture of CO2.en_UK
dc.identifier.citationRusso G, Prpich G, Anthony EJ, (2017) Selective-exhaust gas recirculation for CO2 capture using membrane technology, Journal of Membrane Science, Volume 549, March 2018, pp. 649-659en_UK
dc.identifier.issn0376-7388
dc.identifier.urihttps://doi.org/10.1016/j.memsci.2017.10.052
dc.identifier.urihttp://dspace.lib.cranfield.ac.uk/handle/1826/12716
dc.language.isoenen_UK
dc.publisherElsevieren_UK
dc.rightsAttribution-NonCommercial-NoDerivatives 4.0 International
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.titleSelective-exhaust gas recirculation for CO2 capture using membrane technologyen_UK
dc.typeArticleen_UK

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